In Situ Formed Tribofilms as Efficient Organic/Inorganic Hybrid Interlayers for Stabilizing Lithium Metal Anodes

In Situ Formed Tribofilms as Efficient Organic/Inorganic Hybrid Interlayers for Stabilizing Lithium Metal Anodes

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Highlights The robust organic/inorganic hybrid interlayer derived from in situ formed tribofilms REVITALIZING SHAMPOO were fabricated by using a scalable rolling method.The interlayer facilitates dendrite-free lithium metal anodes by building local de-solvation environments near the interface and inhibiting both dendrite Mystery Box growth and electrolytes corrosion.The symmetrical cell exhibits a remarkable lifespan of 5,600 h (1.0 mA cm-2 and 1.

0 mAh cm-2) and 1,350 cycles even at a harsh condition (18.0 mA cm-2 and 3.0 mAh cm-2).